Structural organization of the human eukaryotic initiation factor 5A precursor and its site-directed variant Lys50-->Arg

Amino Acids. 1999;16(1):91-106. doi: 10.1007/BF01318888.

Abstract

The molecular properties of the human eukaryotic initiation factor 5A precursor and its site directed Lys50-->Arg variant have been investigated and compared. Structure perturbation methods were used to gain information about the protein architecture in solution. Intrinsic and extrinsic spectroscopic probes strategically located in the protein matrix detected the independent unfolding of two molecular regions. Three cysteines out of four were titrated in the native protein and the peculiar presence of a tyrosinate band at neutral pH was detected. At alkaline pH only two tyrosines out of three were titratable in the native protein, with an apparent pK of about 9.9. Native protein and its Lys50-->Arg variant reacted in a similar fashion to guanidine and to pH variation, but differently to thermal stress. The complex thermal unfolding of both proteins indicated the presence of intermediates. Spectroscopic data showed that these intermediates are differently structured. Consequently, the two proteins seem to have different unfolding pathways.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Substitution
  • Arginine / chemistry*
  • Base Sequence
  • Circular Dichroism
  • DNA Primers
  • Eukaryotic Translation Initiation Factor 5A
  • Fluorescent Dyes
  • Guanidine / chemistry
  • Humans
  • Lysine / chemistry*
  • Mutagenesis, Site-Directed
  • Naphthalenesulfonates
  • Peptide Initiation Factors / chemistry*
  • Peptide Initiation Factors / genetics
  • Protein Conformation
  • Protein Denaturation
  • Protein Precursors / chemistry*
  • Protein Precursors / genetics
  • RNA-Binding Proteins*
  • Spectrophotometry, Ultraviolet

Substances

  • DNA Primers
  • Fluorescent Dyes
  • Naphthalenesulfonates
  • Peptide Initiation Factors
  • Protein Precursors
  • RNA-Binding Proteins
  • 1,5-I-AEDANS
  • Arginine
  • Guanidine
  • Lysine