Studies of the novel ketolide ABT-773: transport, binding to ribosomes, and inhibition of protein synthesis in Streptococcus pneumoniae

Antimicrob Agents Chemother. 2000 Jun;44(6):1562-7. doi: 10.1128/AAC.44.6.1562-1567.2000.

Abstract

Macrolide resistance in Streptococcus pneumoniae has been associated with two main mechanisms: target modification by Erm methyltransferases and efflux by macrolide pumps. The ketolide ABT-773, which has a 3-keto group and no L-cladinose sugar, represents a new class of drugs with in vitro activity against a variety of resistant bacteria. Several approaches were undertaken to understand how ABT-773 was able to defeat resistance mechanisms. We demonstrated tighter ribosome binding of ABT-773 than erythromycin. We also showed that ABT-773 (i) accumulated in macrolide-sensitive S. pneumoniae at a higher rate than erythromycin, (ii) was able to bind with methylated ribosomes, though at lower affinities than with wild-type ribosomes, and (iii) accumulated in S. pneumoniae strains with the efflux-resistant phenotype.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anti-Bacterial Agents / pharmacology
  • Bacterial Proteins / biosynthesis
  • Biological Transport
  • Drug Resistance, Microbial
  • Erythromycin / analogs & derivatives*
  • Erythromycin / pharmacology
  • Ketolides*
  • Ribosomes / drug effects
  • Streptococcus pneumoniae / drug effects*
  • Streptococcus pneumoniae / metabolism

Substances

  • Anti-Bacterial Agents
  • Bacterial Proteins
  • Ketolides
  • Erythromycin
  • cethromycin