Preclinical antitumor activity of BMS-214662, a highly apoptotic and novel farnesyltransferase inhibitor

Cancer Res. 2001 Oct 15;61(20):7507-17.

Abstract

BMS-214662 is a potent and selective inhibitor of farnesyltransferase (FTI). In rodent fibroblasts transformed by oncogenes, BMS-214662 reversed the H-Ras-transformed phenotype but not that of K-Ras or other oncogenes. In soft agar growth assays, BMS-214662 showed good potency in inhibiting H-ras-transformed rodent cells, A2780 human ovarian carcinoma tumor cells, and HCT-116 human colon carcinoma tumor cells. Inhibition of H-Ras processing in HCT-116 human colon tumor cells was more rapid than in H-Ras-transformed rodent fibroblast tumors. BMS-214662 is the most potent apoptotic FTI known and demonstrated broad spectrum yet robust cell-selective cytotoxic activity against a panel of cell lines with diverse histology. The presence of a mutant ras oncogene was not a prerequisite for sensitivity. Athymic and conventional mice were implanted s.c. with different histological types of human and murine tumors, respectively. BMS-214662 was administered both parenterally and p.o. and was active by all these routes. Curative responses were observed in mice bearing staged human tumor xenografts including HCT-116 and HT-29 colon, MiaPaCa pancreatic, Calu-1 lung, and EJ-1 bladder carcinomas. A subline of HCT-116, HCT-116/VM46, resistant to many standard cytotoxic agents by means of a multiple drug resistance mechanism, remained quite susceptible to BMS-214662, and borderline activity was achieved against N-87 human gastric carcinoma. Two murine tumors, Lewis lung carcinoma and M5076 sarcoma, were insensitive to the FTI. In a study performed using Calu-1 tumor-bearing mice, no obvious schedule dependency of BMS-214662 was observed. The FTI, BMS-214662, demonstrated broad spectrum activity against human tumors, but murine tumors were not as sensitive.

MeSH terms

  • Alkyl and Aryl Transferases / antagonists & inhibitors*
  • Animals
  • Antineoplastic Agents / pharmacology*
  • Antineoplastic Agents / toxicity
  • Apoptosis / drug effects*
  • Benzodiazepines / pharmacology*
  • Benzodiazepines / toxicity
  • Cattle
  • Drug Administration Schedule
  • Drug Screening Assays, Antitumor
  • Enzyme Inhibitors / pharmacology*
  • Enzyme Inhibitors / toxicity
  • Farnesyltranstransferase
  • Humans
  • Imidazoles / pharmacology*
  • Imidazoles / toxicity
  • Mice
  • Mice, Inbred C57BL
  • Mice, Inbred DBA
  • Neoplasms / drug therapy
  • Neoplasms / pathology
  • Neoplasms, Experimental / drug therapy
  • Neoplasms, Experimental / pathology
  • Xenograft Model Antitumor Assays
  • ras Proteins / antagonists & inhibitors
  • ras Proteins / metabolism

Substances

  • Antineoplastic Agents
  • Enzyme Inhibitors
  • Imidazoles
  • Benzodiazepines
  • Alkyl and Aryl Transferases
  • Farnesyltranstransferase
  • ras Proteins
  • 7-cyano-2,3,4,5-tetrahydro-1-(1H-imidazol-4-ylmethyl)-3-(phenylmethyl)-4-(2-thienylsulfonyl)-1H-1,4-benzodiazepine