Design and synthesis of a template-assembled oligomannose cluster as an epitope mimic for human HIV-neutralizing antibody 2G12

Org Biomol Chem. 2004 Feb 21;2(4):483-8. doi: 10.1039/b314565d. Epub 2004 Jan 22.

Abstract

The synthesis and antibody-binding affinity of a novel template-assembled oligomannose cluster as an epitope mimic for human anti-HIV antibody 2G12 are described. Cholic acid was chosen as the scaffold and three high-mannose type oligosaccharide (Man(9)GlcNAc(2)Asn) moieties were selectively attached at the 3alpha, 7alpha, and 12alpha-positions of the scaffold through a series of regioselective transformations. Binding studies revealed that the synthetic oligosaccharide cluster is 46-fold more effective than the subunit Man(9)GlcNAc(2)Asn in inhibiting 2G12-binding to immobilized gp120. The scaffold approach described in this paper provides an avenue to designing more effective epitope mimics for antibody 2G12 in the hope of developing a carbohydrate-based vaccine against HIV-1.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Antibodies, Monoclonal / chemistry*
  • Antibodies, Neutralizing / chemistry*
  • Biomimetic Materials / chemistry*
  • Broadly Neutralizing Antibodies
  • Drug Design
  • Epitopes / chemistry*
  • HIV Antibodies / chemistry*
  • Mannose / chemistry*
  • Models, Molecular
  • Molecular Structure
  • Oligosaccharides / chemical synthesis*

Substances

  • 2G12 monoclonal antibody
  • Antibodies, Monoclonal
  • Antibodies, Neutralizing
  • Broadly Neutralizing Antibodies
  • Epitopes
  • HIV Antibodies
  • Oligosaccharides
  • Mannose