Lipoxins and novel 15-epi-lipoxin analogs display potent anti-inflammatory actions after oral administration

Br J Pharmacol. 2004 Sep;143(1):43-52. doi: 10.1038/sj.bjp.0705912. Epub 2004 Aug 9.

Abstract

1. Lipoxins (LX) and aspirin-triggered 15-epi-lipoxins (ATL) exert potent anti-inflammatory actions. In the present study, we determined the anti-inflammatory efficacy of endogenous LXA(4) and LXB(4), the stable ATL analog ATLa2, and a series of novel 3-oxa-ATL analogs (ZK-996, ZK-990, ZK-994, and ZK-142) after intravenous, oral, and topical administration in mice. 2. LXA(4), LXB(4), ATLa2, and ZK-994 were orally active, exhibiting potent systemic inhibition of zymosan A-induced peritonitis at very low doses (50 ng kg(-1)-50 microg kg(-1)). 3. Intravenous ZK-994 and ZK-142 (500 microg kg(-1)) potently attenuated hind limb ischemia/reperfusion-induced lung injury, with 32+/-12 and 53+/-5% inhibition (P<0.05), respectively, of neutrophil accumulation in lungs. The same dose of ATLa2 had no significant protective action. 4. Topical application of ATLa2, ZK-994, and ZK-142 ( approximately 20 microg cm(-2)) prevented vascular leakage and neutrophil infiltration in LTB(4)/PGE(2)-stimulated ear skin inflammation. While ATLa2 and ZK-142 displayed approximately equal anti-inflammatory efficacy in this model, ZK-994 displayed a slower onset of action. 5. In summary, native LXA(4) and LXB(4), and analogs ATLa2, ZK-142, and ZK-994 retain broad anti-inflammatory effects after intravenous, oral, and topical administration. The 3-oxa-ATL analogs, which have enhanced metabolic and chemical stability and a superior pharmacokinetic profile, provide new opportunities to explore the actions and therapeutic potential for LX and ATL.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Administration, Topical
  • Animals
  • Anti-Inflammatory Agents, Non-Steroidal / pharmacology*
  • Aspirin / pharmacology
  • Ear, External / pathology
  • Inflammation / pathology
  • Inflammation / prevention & control
  • Injections, Intravenous
  • Lipoxins / administration & dosage
  • Lipoxins / pharmacology*
  • Lung Diseases / pathology
  • Lung Diseases / prevention & control
  • Male
  • Mice
  • Peritonitis / chemically induced
  • Peritonitis / pathology
  • Peritonitis / prevention & control
  • Reperfusion Injury / pathology
  • Reperfusion Injury / prevention & control
  • Zymosan / toxicity

Substances

  • Anti-Inflammatory Agents, Non-Steroidal
  • Lipoxins
  • lipoxin A4
  • Zymosan
  • Aspirin