LC-MS/MS-analysis of prostaglandin E2 and D2 in microdialysis samples of rats

J Chromatogr B Analyt Technol Biomed Life Sci. 2005 Nov 5;826(1-2):188-97. doi: 10.1016/j.jchromb.2005.09.001. Epub 2005 Sep 19.

Abstract

For the determination of prostaglandins in microdialysis samples, usually immunoassays are used. However, these assays may show cross-reactivity among various prostaglandins. To overcome this problem a specific method for the determination of prostaglandin E2 and D2 in rat microdialysis samples by using liquid chromatography-electrospay ionization-tandem mass spectrometry (LC-ESI-MS/MS) is described. Prostaglandin E2 and D2 were extracted from microdialysis samples with liquid-liquid extraction using deuterated prostaglandin D2, [2H4]-PGD2, as internal standard. Subsequently, prostaglandins were separated with a phenomenex Synergi Hydro-RP column and determined with a PE Sciex API 3000 mass spectrometer equipped with a turbo ion spray interface operating in negative ionization mode. The method showed a LLOQ of 25 pg/ml for prostaglandin E2 and 50 pg/ml for prostaglandin D2. The applicability of the method is shown in rat spinal cord microdialysis samples following peripheral nociceptive stimulation.

Publication types

  • Research Support, Non-U.S. Gov't
  • Validation Study

MeSH terms

  • Animals
  • Chromatography, Liquid / methods*
  • Dinoprostone / analysis*
  • Drug Stability
  • Male
  • Mass Spectrometry / methods
  • Microdialysis / methods*
  • Prostaglandin D2 / analysis*
  • Rats
  • Rats, Sprague-Dawley
  • Reproducibility of Results
  • Spinal Cord / chemistry

Substances

  • Dinoprostone
  • Prostaglandin D2