Optical spectra of anionic boron cluster compounds and their utilization for photometric detection

Spectrochim Acta A Mol Biomol Spectrosc. 2006 Oct;65(2):378-86. doi: 10.1016/j.saa.2005.11.014. Epub 2006 Mar 23.

Abstract

The article presents first collection of UV-vis absorption spectra of purely synthetic boron cluster compounds. Single-cage compounds have at least 11 cluster atoms; cobaltadicarboranes consists of 2 substituted 11-vertex bis(dicarbollide) clusters sandwiching the central cobalt atom. Spectrum of any of 18 investigated compounds has absorption maximum between 200 and 210 nm; its molar extinction coefficient is of the order of 10(3)-10(4)L/molcm. Second maximum exists in a spectrum of a single-cage compound if its exo-skeletal substituent absorbs UV-light above 200 nm. Spectra of cobaltadicarbaboranes both bridged and unbridged have pronounced second maxima between 270 and 300 nm. Their molar extinction coefficients range from 10(4) to 10(5)L/molcm. First light absorption minimum is close to 254 nm in spectra with two and more absorption maxima. Several correlations are derived between structure of investigated compounds and their UV-vis absorption spectra.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anions
  • Boron Compounds / analysis
  • Boron Compounds / chemistry*
  • Hydrophobic and Hydrophilic Interactions
  • Models, Molecular
  • Molecular Structure
  • Osmolar Concentration
  • Sensitivity and Specificity
  • Solubility
  • Solvents
  • Spectrophotometry, Ultraviolet*

Substances

  • Anions
  • Boron Compounds
  • Solvents