Cyclocarbopalladation of alkynes: a stereoselective method for preparing dibenzoxapine containing tetrasubstituted exocyclic alkenes

Org Lett. 2006 Apr 13;8(8):1685-8. doi: 10.1021/ol060289a.

Abstract

[reaction: see text] A palladium-catalyzed cascade carbometalation-cross coupling of alkyne route was developed for the preparation of tetrasubstituted exocyclic alkenes with high stereo- and regiocontrol. The effectiveness of this novel methodology was demonstrated by the synthesis of a number of dibenzoxapines in sufficient quantities to support their further development.

MeSH terms

  • Alkenes / chemical synthesis*
  • Alkenes / chemistry
  • Alkynes / chemistry*
  • Benzoxepins / chemical synthesis*
  • Combinatorial Chemistry Techniques*
  • Cyclization
  • Molecular Structure
  • Palladium / chemistry

Substances

  • Alkenes
  • Alkynes
  • Benzoxepins
  • Palladium