Charge inversion at high ionic strength studied by streaming currents

Phys Rev Lett. 2006 Jun 9;96(22):224502. doi: 10.1103/PhysRevLett.96.224502. Epub 2006 Jun 6.

Abstract

We report charge inversion, the sign reversal of the effective surface charge in the presence of multivalent counterions, for the biologically relevant regimes of divalent ions and mixtures of monovalent and multivalent ions. Using streaming currents, the pressure-driven transport of countercharges in the diffuse layer, we find that charge inversion occurs in rectangular silica nanochannels at high concentrations of divalent ions. Strong monovalent screening is found to cancel charge inversion, restoring the original surface charge polarity. An analytical model based on ion correlations successfully describes our observations.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Ion Channels / chemistry*
  • Ions / chemistry*
  • Models, Chemical*
  • Nanostructures / chemistry*
  • Osmolar Concentration
  • Silicon Dioxide / chemistry

Substances

  • Ion Channels
  • Ions
  • Silicon Dioxide