Electrochemical proteolytic beacon for detection of matrix metalloproteinase activities

J Am Chem Soc. 2006 Sep 27;128(38):12382-3. doi: 10.1021/ja0626638.

Abstract

This communication describes a novel method for detecting matrix metalloproteinase-7 activity using a peptide substrate labeled with a ferrocene reporter. The substrate serves as a selective "electrochemical proteolytic beacon" (EPB) for this metalloproteinase. The EPB is immobilized on a gold electrode surface to enable "on-off" electrochemical signaling capability for uncleaved and cleaved events. The EPB is efficiently and selectively cleaved by MMP-7 as measured by the rate of decrease in redox current of ferrocene. Direct transduction of a signal corresponding to peptide cleavage events into an electronic signal thus provides a simple, sensitive route for detecting the MMP activity. The new method allows for identification of the activity of MMP-7 in concentrations as low as 3.4 pM. The concept can be extended to design a multiple peptide substrate labeled with different electroactive reporters for assaying multiple MMPs activities.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Electrochemistry
  • Ferrous Compounds / chemistry*
  • Matrix Metalloproteinase 7 / chemistry*
  • Matrix Metalloproteinase 7 / metabolism*
  • Metallocenes
  • Oligopeptides / chemical synthesis
  • Oligopeptides / chemistry*
  • Oligopeptides / metabolism
  • Protein Structure, Secondary

Substances

  • Ferrous Compounds
  • Metallocenes
  • Oligopeptides
  • Matrix Metalloproteinase 7
  • ferrocene