Radiosensitization by 2-benzoyl-3-phenyl-6,7-dichloroquinoxaline 1,4-dioxide under oxia and hypoxia in human colon cancer cells

Radiat Oncol. 2007 Jan 3:2:1. doi: 10.1186/1748-717X-2-1.

Abstract

Background: The sensitizing effects of 2-benzoyl-3-phenyl-6,7-dichloroquinoxaline 1,4-dioxide (DCQ) and ionizing radiation (IR) were determined in four colon cancer cells and in FHs74Int normal intestinal cells.

Methods: Cell cycle modulation, TUNEL assay, clonogenic survival and DNA damage were examined under oxia or hypoxia. Effects on apoptotic molecules and on p-Akt and Cox-2 protein expression were investigated.

Results: The four cell lines responded differently to DCQ+IR; HT-29 cells were most resistant. Combination treatment caused significant increases in preG1 (apoptosis) in HCT-116, while G2/M arrest occurred in DLD-1. DCQ potentiated IR effects more so under hypoxia than oxia. Pre-exposure of DLD-1 to hypoxia induced 30% apoptosis, and G2/M arrest in oxia. The survival rate was 50% lower in DCQ+IR than DCQ alone and this rate further decreased under hypoxia. FHs74Int normal intestinal cells were more resistant to DCQ+IR than cancer cells.Greater ssDNA damage occurred in DLD-1 exposed to DCQ+IR under hypoxia than oxia. In oxia, p-Akt protein expression increased upon IR exposure and drug pre-treatment inhibited this increase. In contrast, in hypoxia, exposure to IR reduced p-Akt protein and DCQ restored its expression to the untreated control. Apoptosis induced in hypoxic DLD-1 cells was independent of p53-p21 modulation but was associated with an increase in Bax/Bcl-2 ratio and the inhibition of the Cox-2 protein.

Conclusion: DCQ is a hypoxic cell radiosensitizer in DLD-1 human colon cancer cells.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Apoptosis
  • Cell Cycle
  • Cell Line, Tumor
  • Colonic Neoplasms / pathology*
  • Colonic Neoplasms / radiotherapy*
  • Comet Assay
  • DNA Damage
  • Flow Cytometry / methods
  • Humans
  • Hypoxia*
  • In Situ Nick-End Labeling
  • Intestines / drug effects
  • Oxygen / metabolism*
  • Quinoxalines / pharmacology*
  • Radiation Oncology / methods*
  • Radiation-Sensitizing Agents / pharmacology*

Substances

  • 2-benzoyl-3-phenyl-6,7-dichloroquinoxaline-1,4-dioxide
  • Quinoxalines
  • Radiation-Sensitizing Agents
  • Oxygen