F-16438s, novel binding inhibitors of CD44 and hyaluronic acid. I. Establishment of an assay method and biological activity

J Antibiot (Tokyo). 2006 Dec;59(12):770-6. doi: 10.1038/ja.2006.101.

Abstract

In an attempt to obtain inhibitors of hyaluronic acid (HA) binding to its receptor, CD44, we established an efficient assay method to detect and quantify binding using fluorescein-labeled HA and HEK293 cells stably expressing CD44. As a result of the screening of culture broths of microorganisms, we found fungus strain Gloeoporus dichrous SANK 30502 produced inhibitory activity in this new assay. Five compounds, F-16438 A, B, E, F and G, were isolated from the fermentation broths, and their IC50 values were determined to be 10.3, 13.5, 27.3, 12.0 and 13.0 microM, respectively. F-16438 A, B, E, F and G are the first reported inhibitors of binding HA to CD44. F-16438 A, B, E and F have novel structures.

MeSH terms

  • Cell Line
  • Endocytosis
  • Humans
  • Hyaluronan Receptors / metabolism*
  • Hyaluronic Acid / antagonists & inhibitors*
  • Hyaluronic Acid / metabolism
  • Mannosides / pharmacology*
  • Polyporales / metabolism*
  • Salicylates / pharmacology*

Substances

  • Hyaluronan Receptors
  • Mannosides
  • Salicylates
  • Hyaluronic Acid