Characterization of (13C24) T-2 toxin and its use as an internal standard for the quantification of T-2 toxin in cereals with HPLC-MS/MS

Anal Bioanal Chem. 2007 Oct;389(3):931-40. doi: 10.1007/s00216-007-1493-7. Epub 2007 Aug 1.

Abstract

In this paper, the structure and the identity of fully 13C-substituted T-2 toxin were confirmed using high-resolution mass spectrometry, 1H-NMR, 13C-NMR, tandem mass spectrometry and HPLC-DAD. The purity of this compound was estimated to be at least 98.8% according to UV data. The isotopic distribution of (13C(24)) T-2 toxin indicated a total isotopic enrichment of 98.2 +/- 1.0 atom% 13C, and the application of different MS measurement modes revealed the MS/MS fragmentation pattern of T-2 toxin. Furthermore, a stable isotope dilution mass spectrometry method for the quantification of T-2 toxin was developed using (13C(24)) T-2 toxin as internal standard. The method was evaluated with and without conventional clean-up and validated for maize and oats. Both cereals showed strong matrix enhancement effects, which could be compensated for through the application of the isotope-substituted internal standard.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Avena / chemistry
  • Carbon Isotopes / analysis*
  • Carbon Isotopes / chemistry
  • Chromatography, High Pressure Liquid / methods*
  • Chromatography, High Pressure Liquid / standards
  • Edible Grain / chemistry*
  • Mass Spectrometry / methods*
  • Mass Spectrometry / standards
  • Radioisotope Dilution Technique
  • Reproducibility of Results
  • Sensitivity and Specificity
  • T-2 Toxin / analysis*
  • Zea mays / chemistry

Substances

  • Carbon Isotopes
  • T-2 Toxin