Quantification of cyclosporine and tacrolimus in whole blood. Comparison of liquid chromatography-electrospray mass spectrometry with the enzyme multiplied immunoassay technique

Clin Biochem. 2008 Jul;41(10-11):910-3. doi: 10.1016/j.clinbiochem.2008.02.015. Epub 2008 Mar 12.

Abstract

Objectives: The aim of this work was to compare a validated liquid chromatography-mass spectrometry (LC-MS) method with the commercial enzyme multiplied immunoassay technique (EMIT) for cyclosporine and tacrolimus whole blood quantification.

Design and methods: Samples of transplant patients receiving cyclosporine (n=38) or tacrolimus (n=41) were analyzed successively by LC-MS and EMIT. Several statistical approaches for method comparison were evaluated and Passing-Bablok and Bland-Altman analyses chosen.

Results: Overestimations of the concentrations measured with EMIT compared to LC-MS were observed with means of 23% (range: 6% to 46%) for cyclosporine and 30% (range: -3% to 73%) for tacrolimus.

Conclusion: The EMIT demonstrated significant positive biases due to cross-reactions with metabolites. This indicates that, in some clinical situations, a selective method such as LC-MS is preferable for therapeutic drug monitoring in transplant patients.

MeSH terms

  • Cross Reactions
  • Cyclosporine / blood*
  • Enzyme Multiplied Immunoassay Technique
  • Humans
  • Immunoassay
  • Spectrometry, Mass, Electrospray Ionization / methods
  • Tacrolimus / blood*
  • Transplantation Immunology

Substances

  • Cyclosporine
  • Tacrolimus