Anti-oxidant treatment enhances anti-tumor cytotoxicity of (-)-gossypol

Cancer Biol Ther. 2008 May;7(5):767-76. doi: 10.4161/cbt.7.5.5767. Epub 2008 May 20.

Abstract

We showed that tumor cells with wild-type p53 and high levels of Bcl-x(L) are cisplatin resistant but are induced to undergo apoptosis by (-)-gossypol, making this a promising agent for overcoming cisplatin resistance. However, some cells in a population with this phenotype are not killed and continue to survive. Conversely, tumor cells with low Bcl-x(L) expression and either wild type or mutant p53 are relatively cisplatin sensitive and do not exhibit such high levels of apoptosis. However, these do undergo progressive loss of viability after (-)-gossypol that may not be tumor specific. We sought to elucidate the basis for these observations using cDNA microarray analysis of (-)-gossypol treated cisplatin sensitive and resistant cells. Genes in the reactive oxygen species (ROS) pathway were highly upregulated in response to (-)-gossypol. The upregulation was of much greater magnitude in cisplatin sensitive than resistant cells. Staining with an oxidation reporter dye confirmed differential induction of ROS in tumor cells with low Bcl-x(L). As (-)-gossypol is known to undergo oxidative metabolism in vivo, ROS generation may be responsible for both off-target cytotoxicity and inactivation of the drug. In agreement with this hypothesis, oxidation of (-)-gossypol by pre-treatment with hydrogen peroxide eliminated its activity. Combined treatment with the antioxidant N-acetyl-cysteine (NAC) to block ROS increased (-)-gossypol-induced cytotoxicity to tumor but not normal cells. Furthermore, NAC increased the induction of apoptosis as measured by the sub-G(1) population, in both cisplatin sensitive and resistant cells. We postulate that concurrent treatment with antioxidant to block ROS prevents oxidative inactivation of (-)-gossypol and limits off-target toxicity allowing more potent (-)-gossypol-induced anti-tumor activity.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Acetylcysteine / pharmacology
  • Antineoplastic Agents / pharmacology*
  • Antioxidants / pharmacology*
  • Cell Line
  • Cell Line, Tumor
  • Cell Survival
  • Drug Synergism
  • Gene Expression Regulation, Neoplastic*
  • Gossypol / pharmacology*
  • Humans
  • Models, Biological
  • Neoplasms / drug therapy*
  • Oligonucleotide Array Sequence Analysis
  • Oxidants / metabolism
  • Reactive Oxygen Species

Substances

  • Antineoplastic Agents
  • Antioxidants
  • Oxidants
  • Reactive Oxygen Species
  • Gossypol
  • Acetylcysteine