Development of a homogeneous high-throughput live-cell G-protein-coupled receptor binding assay

J Biomol Screen. 2008 Sep;13(8):748-54. doi: 10.1177/1087057108317835. Epub 2008 May 6.

Abstract

The measurement of ligand receptor binding parameters for G-protein-coupled receptors is indispensable in the drug discovery process. Traditional ligand receptor binding assays require scale-up of cells and membrane preparations, which is an expensive and time-consuming process. In this report, the authors describe the development of a homogeneous live-cell binding assay for GPCRs using a fluorophore-labeled nonpeptide ligand. The model assay used Cy3B-labeled telenzepine and Chinese hamster ovary cells expressing M1 muscarinic acetylcholine receptors. This homogeneous live-cell fluorescence binding assay format is superior to the traditional binding methods because it measures binding of a ligand to intact receptors on living cells. The assay requires no washing or separation steps, thereby allowing a real-time kinetic readout for the determination of ligand association and dissociation from the intact receptors. The results also suggest that miniaturization is feasible without compromising the data quality.

MeSH terms

  • Animals
  • Atropine / metabolism
  • Benzenesulfonates / metabolism
  • Biological Assay / methods*
  • CHO Cells
  • Carbocyanines / metabolism
  • Cricetinae
  • Cricetulus
  • Fluorescent Dyes / metabolism
  • Ligands
  • Miniaturization
  • Muscarinic Antagonists / chemistry
  • Muscarinic Antagonists / metabolism
  • Parasympatholytics / metabolism
  • Pirenzepine / analogs & derivatives
  • Pirenzepine / metabolism
  • Quinuclidinyl Benzilate / chemistry
  • Quinuclidinyl Benzilate / metabolism
  • Receptor, Muscarinic M1 / metabolism
  • Receptors, G-Protein-Coupled / genetics
  • Receptors, G-Protein-Coupled / metabolism*

Substances

  • Benzenesulfonates
  • Carbocyanines
  • Cy3B N-hydroxysuccinimide ester
  • Fluorescent Dyes
  • Ligands
  • Muscarinic Antagonists
  • Parasympatholytics
  • Receptor, Muscarinic M1
  • Receptors, G-Protein-Coupled
  • telenzepine
  • Pirenzepine
  • Quinuclidinyl Benzilate
  • Atropine