Membrane-bound pyrroloquinoline quinone-dependent dehydrogenase in Gluconobacter oxydans M5, responsible for production of 6-(2-hydroxyethyl) amino-6-deoxy-L-sorbose

Appl Environ Microbiol. 2008 Aug;74(16):5250-3. doi: 10.1128/AEM.00272-08. Epub 2008 May 23.

Abstract

A membrane-bound protein purified from Gluconobacter oxydans M5 was confirmed to be a pyrroloquinoline quinone-dependent D-sorbitol dehydrogenase. Gene disruption and complementation experiments demonstrated that this enzyme is responsible for the oxidation of 1-(2-hydroxyethyl) amino-1-deoxy-D-sorbitol (1NSL) to 6-(2-hydroxyethyl) amino-6-deoxy-L-sorbose (6NSE), which is the precursor of an antidiabetic drug, miglitol.

MeSH terms

  • Amino Acid Sequence
  • Bacterial Proteins / isolation & purification
  • Bacterial Proteins / metabolism*
  • Genetic Complementation Test
  • Genetic Vectors
  • Gluconobacter oxydans / enzymology*
  • Gluconobacter oxydans / genetics
  • L-Iditol 2-Dehydrogenase / isolation & purification
  • L-Iditol 2-Dehydrogenase / metabolism*
  • Membrane Proteins / metabolism
  • Oxidation-Reduction
  • PQQ Cofactor / metabolism*
  • Plasmids
  • Sorbitol / metabolism
  • Sorbose / analogs & derivatives*
  • Sorbose / biosynthesis*

Substances

  • 6-(2-hydroxyethyl) amino-6-deoxy-L-sorbose
  • Bacterial Proteins
  • Membrane Proteins
  • Sorbitol
  • PQQ Cofactor
  • L-Iditol 2-Dehydrogenase
  • Sorbose