Influence of xanthine oxidase on thiopurine metabolism in Crohn's disease

Aliment Pharmacol Ther. 2008 Sep 15;28(6):749-57. doi: 10.1111/j.1365-2036.2008.03768.x.

Abstract

Background: The thiopurines, azathioprine (AZA) and mercaptopurine are extensively used in Crohn's discase (CD). Thiopurine bioactivation can be diverted by either thiopurine methyltransferase (TPMT), or by xanthine oxidase/dehydrogenase (XOD) which forms 6-thiouric acid (6TU).

Aim: To investigate whether chronic inflammation could influence small intestinal XOD activity using urinary excretion of 6TU as a surrogate marker of XOD activity.

Methods: 6-Thiouric acid excretion was compared between 32 CD patients and nine dermatology patients (control group), on AZA. Six CD patients were interesting: five with low TPMT activity (one deficient, four intermediate), and one receiving AZA/allopurinol co-therapy.

Results: There was no statistical difference in 6TU excretion between the CD and control group. CD location, severity or surgery did not affect excretion. The TPMT-deficient patient excreted 89% of daily AZA dose as 6TU, but excretion by TPMT carriers was essentially normal. Concurrent 5-aminosalicylic acid therapy increased 6TU excretion significantly (median 32.9%), consistent with inhibiting TPMT. 6TU was undetectable in the patient on AZA/allopurinol co-therapy.

Conclusions: The results refuted our hypothesis, but fitted a model where most of an oral thiopurine dose effectively escapes first-pass metabolism by gut XOD, but is heavily catabolized by TPMT. Bioavailability of thiopurines may be competitively inhibited by dietary purines.

Publication types

  • Case Reports

MeSH terms

  • Adult
  • Biological Availability
  • Case-Control Studies
  • Crohn Disease / drug therapy*
  • Crohn Disease / enzymology
  • Crohn Disease / pathology
  • Female
  • Humans
  • Immunosuppressive Agents / metabolism*
  • Intestine, Small / enzymology
  • Mercaptopurine / analogs & derivatives*
  • Mercaptopurine / metabolism
  • Methyltransferases / genetics
  • Methyltransferases / metabolism
  • Uric Acid / analogs & derivatives*
  • Uric Acid / urine
  • Xanthine Oxidase / metabolism*

Substances

  • Immunosuppressive Agents
  • azathiopurine
  • Uric Acid
  • 6-thiouric acid
  • Mercaptopurine
  • Xanthine Oxidase
  • Methyltransferases
  • thiopurine methyltransferase