4-Aminobiphenyl downregulation of NAT2 acetylator genotype-dependent N- and O-acetylation of aromatic and heterocyclic amine carcinogens in primary mammary epithelial cell cultures from rapid and slow acetylator rats

Toxicol Sci. 2009 Jan;107(1):293-7. doi: 10.1093/toxsci/kfn216. Epub 2008 Oct 8.

Abstract

Aromatic and heterocyclic amine carcinogens present in the diet and in cigarette smoke induce breast tumors in rats. N-acetyltransferase 1 (NAT1) and N-acetyltransferase 2 (NAT2) enzymes have important roles in their metabolic activation and deactivation. Human epidemiological studies suggest that genetic polymorphisms in NAT1 and/or NAT2 modify breast cancer risk in women exposed to these carcinogens. p-Aminobenzoic acid (selective for rat NAT2) and sulfamethazine (SMZ; selective for rat NAT1) N-acetyltransferase catalytic activities were both expressed in primary cultures of rat mammary epithelial cells. PABA, 2-aminofluorene, and 4-aminobiphenyl N-acetyltransferase and N-hydroxy-2-amino-1-methyl-6-phenylimidazo[4,5-b] pyridine and N-hydroxy-2-amino-3,8-dimethylimidazo[4,5-f]quinoxaline O-acetyltransferase activities were two- to threefold higher in mammary epithelial cell cultures from rapid than slow acetylator rats. In contrast, SMZ (a rat NAT1-selective substrate) N-acetyltransferase activity did not differ between rapid and slow acetylators. Rat mammary cells cultured in the medium supplemented 24 h with 10muM ABP showed downregulation in the N-and O-acetylation of all substrates tested except for the NAT1-selective substrate SMZ. This downregulation was comparable in rapid and slow NAT2 acetylators. These studies clearly show NAT2 acetylator genotype-dependent N- and O-acetylation of aromatic and heterocyclic amine carcinogens in rat mammary epithelial cell cultures to be subject to downregulation by the arylamine carcinogen ABP.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • 4-Aminobenzoic Acid / metabolism
  • Acetylation*
  • Aminobiphenyl Compounds / metabolism*
  • Animals
  • Arylamine N-Acetyltransferase / genetics
  • Arylamine N-Acetyltransferase / metabolism*
  • Carcinogens / metabolism*
  • Cells, Cultured
  • Down-Regulation / genetics*
  • Fluorenes
  • Gene Expression Regulation, Enzymologic / physiology
  • Humans
  • Isoenzymes / genetics
  • Isoenzymes / metabolism
  • Mammary Glands, Animal
  • Polymorphism, Genetic
  • Rats
  • Sulfamethazine / metabolism

Substances

  • Aminobiphenyl Compounds
  • Carcinogens
  • Fluorenes
  • Isoenzymes
  • 4-biphenylamine
  • 2-aminofluorene
  • Sulfamethazine
  • Arylamine N-Acetyltransferase
  • N-acetyltransferase 1
  • 4-Aminobenzoic Acid