Enzymatic diagnosis of Sjögren-Larsson syndrome using electrospray ionization mass spectrometry

J Chromatogr B Analyt Technol Biomed Life Sci. 2009 Feb 1;877(4):451-5. doi: 10.1016/j.jchromb.2008.12.040. Epub 2008 Dec 25.

Abstract

Background: Sjögren-Larsson syndrome is a metabolic disorder characterized by accumulation of long-chain fatty alcohols in plasma of patients due to mutations in the ALDH3A2 gene, that codes for a microsomal fatty aldehyde dehydrogenase (FALDH). Recent studies have demonstrated that FALDH is involved in the last step of the conversion of 22-hydroxy-C22:0 into the dicarboxylic acid of C22:0 (C22:0-DCA).

Methods: FALDH activity was determined by incubating fibroblast homogenates with omega-hydroxy-C22:0 in the presence of NAD(+). Electrospray ionization mass spectrometry (ESI-MS) was used to quantify the amounts of C22:0-DCA produced.

Results: All SLS patients were deficient in C22:0-DCA productions with activities ranging from 3.2-26.3% of mean control.

Conclusions: The new assay described in this paper has substantial advantages over previous assays, and allows for the easy, reliable and rapid diagnosis of SLS.

Publication types

  • Research Support, Non-U.S. Gov't
  • Validation Study

MeSH terms

  • Aldehyde Oxidoreductases / genetics*
  • Humans
  • Sjogren-Larsson Syndrome / diagnosis*
  • Sjogren-Larsson Syndrome / enzymology
  • Sjogren-Larsson Syndrome / genetics
  • Spectrometry, Mass, Electrospray Ionization / methods*

Substances

  • Aldehyde Oxidoreductases
  • long-chain-aldehyde dehydrogenase