D-amino acids govern stationary phase cell wall remodeling in bacteria

Science. 2009 Sep 18;325(5947):1552-5. doi: 10.1126/science.1178123.

Abstract

In all known organisms, amino acids are predominantly thought to be synthesized and used as their L-enantiomers. Here, we found that bacteria produce diverse D-amino acids as well, which accumulate at millimolar concentrations in supernatants of stationary phase cultures. In Vibrio cholerae, a dedicated racemase produced D-Met and D-Leu, whereas Bacillus subtilis generated D-Tyr and D-Phe. These unusual D-amino acids appear to modulate synthesis of peptidoglycan, a strong and elastic polymer that serves as the stress-bearing component of the bacterial cell wall. D-Amino acids influenced peptidoglycan composition, amount, and strength, both by means of their incorporation into the polymer and by regulating enzymes that synthesize and modify it. Thus, synthesis of D-amino acids may be a common strategy for bacteria to adapt to changing environmental conditions.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alanine / chemistry
  • Alanine / metabolism
  • Amino Acid Isomerases / genetics
  • Amino Acid Isomerases / metabolism
  • Amino Acids / chemistry
  • Amino Acids / metabolism*
  • Bacillus subtilis / growth & development
  • Bacillus subtilis / metabolism*
  • Bacillus subtilis / ultrastructure
  • Cell Wall / metabolism*
  • Cell Wall / ultrastructure
  • Down-Regulation
  • Glutamic Acid / chemistry
  • Glutamic Acid / metabolism
  • Isoleucine / metabolism
  • Leucine / metabolism
  • Methionine / metabolism
  • Oligopeptides / chemistry
  • Peptidoglycan / biosynthesis*
  • Peptidoglycan / chemistry
  • Polysaccharides / chemistry
  • Stereoisomerism
  • Valine / metabolism
  • Vibrio cholerae / cytology
  • Vibrio cholerae / growth & development
  • Vibrio cholerae / metabolism*
  • Vibrio cholerae / ultrastructure

Substances

  • Amino Acids
  • Oligopeptides
  • Peptidoglycan
  • Polysaccharides
  • Isoleucine
  • Glutamic Acid
  • Methionine
  • Amino Acid Isomerases
  • Leucine
  • Valine
  • Alanine