A novel pharmacophore model for the design of anthrax lethal factor inhibitors

Chem Biol Drug Des. 2010 Sep 1;76(3):263-8. doi: 10.1111/j.1747-0285.2010.01000.x. Epub 2010 Jun 21.

Abstract

This study aims at the identification of novel structural features on the surface of the Zn-dependent metalloprotease lethal factor (LF) from anthrax onto which to design novel and selective inhibitors. We report that by targeting an unexplored region of LF that exhibits ligand-induced conformational changes, we could obtain inhibitors with at least 30-fold LF selectivity compared to two other most related human metalloproteases, MMP-2 and MMP-9. Based on these results, we propose a novel pharmacophore model that, together with the preliminarily identified compounds, should help the design of more potent and selective inhibitors against anthrax.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Anthrax / drug therapy
  • Antigens, Bacterial / chemistry
  • Bacterial Toxins / antagonists & inhibitors*
  • Bacterial Toxins / chemistry
  • Crystallography, X-Ray
  • Drug Evaluation, Preclinical
  • Enzyme Inhibitors / chemistry*
  • Humans
  • Metalloproteases / antagonists & inhibitors
  • Metalloproteases / chemistry
  • Models, Molecular
  • Structure-Activity Relationship

Substances

  • Antigens, Bacterial
  • Bacterial Toxins
  • Enzyme Inhibitors
  • anthrax toxin
  • Metalloproteases