In vitro assessment of cytochrome P450 inhibition and induction potential of tanespimycin and its major metabolite, 17-amino-17-demethoxygeldanamycin

Cancer Chemother Pharmacol. 2012 Jan;69(1):51-6. doi: 10.1007/s00280-011-1672-2. Epub 2011 May 19.

Abstract

Purpose: To assess the inhibition and induction potential of tanespimycin and its major metabolite, 17-amino-17-demethoxygeldanamycin (17-AG) on cytochrome P450 (CYP) enzymes.

Methods: The inhibitory effect of tanespimycin and 17-AG on various CYP enzymes was determined in human liver microsomes. The inductive effects of tanespimycin and 17-AG on CYP1A2, CYP2B6, and CYP3A4/5 were determined in cultured primary human hepatocytes.

Results: Tanespimycin did not inhibit the activities of CYP1A2, 2A6, 2B6, and 2E1 up to a concentration of 60 μM, while it moderately inhibited CYP3A4/5 and 2C19, and weakly inhibited CYP2C8, 2C9, and 2D6. In addition, its inhibition on CYP3A4/5 was time-dependent. 17-AG moderately inhibited the activities of CYP3A4/5 and CYP2C19, but did not inhibit other CYPs up to a concentration of 30 μM. The inhibition of CYP3A4/5 by 17-AG was not time-dependent. Tanespimycin and 17-AG did not significantly induce the activities of CYP1A2, CYP2B6, or CYP3A4/5 in cultured human hepatocytes at concentrations up to 40 and 20 μM for tanespimycin and 17-AG, respectively.

Conclusions: Tanespimycin together with its active metabolite, 17-AG are moderate inhibitors of CYP3A4/5 and CYP2C19, but not inducers of CYPs. Therefore, co-administration of tanespimycin has the potential to increase the exposure of substrates of CYP2C19 and CYP3A4/5.

MeSH terms

  • Benzoquinones / administration & dosage
  • Benzoquinones / metabolism
  • Benzoquinones / pharmacology*
  • Cells, Cultured
  • Cytochrome P-450 Enzyme Inhibitors*
  • Dose-Response Relationship, Drug
  • Enzyme Induction / drug effects
  • Enzyme Inhibitors / pharmacology*
  • Hepatocytes / drug effects
  • Hepatocytes / enzymology
  • Humans
  • In Vitro Techniques
  • Lactams, Macrocyclic / administration & dosage
  • Lactams, Macrocyclic / metabolism
  • Lactams, Macrocyclic / pharmacology*
  • Microsomes, Liver / drug effects
  • Microsomes, Liver / enzymology
  • Time Factors

Substances

  • 17-amino-17-demethoxygeldanomycin
  • Benzoquinones
  • Cytochrome P-450 Enzyme Inhibitors
  • Enzyme Inhibitors
  • Lactams, Macrocyclic
  • tanespimycin