Valence band circular dichroism in non-magnetic Ag/Ru(0001) at normal emission

J Phys Condens Matter. 2011 Aug 3;23(30):305006. doi: 10.1088/0953-8984/23/30/305006. Epub 2011 Jul 6.

Abstract

For the non-magnetic system of Ag films on Ru(0001), we have measured the circular dichroism of photoelectrons emitted along the surface normal, the geometry typically used in photoemission electron microscopy. Photoemission spectra were acquired from micrometer-sized regions having uniformly thick Ag films on a single, atomically flat Ru terrace. For a single Ag layer, we find a circular dichroism that exceeds 6% at the d-derived band region around 4.5 eV binding energy. The dichroism decreases as the Ag film thickness increases to three atomic layers. We discuss the origin of the circular dichroism in terms of the symmetry lowering that can occur even in normal emission.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Chemistry, Physical / methods*
  • Circular Dichroism
  • Electrons
  • Photochemistry / methods*
  • Photoelectron Spectroscopy / methods
  • Ruthenium / chemistry
  • Silver / chemistry
  • Surface Properties
  • X-Ray Diffraction
  • X-Rays

Substances

  • Silver
  • Ruthenium