Novel suppressive effects of cardamonin on the activity and expression of transglutaminase-2 lead to blocking the migration and invasion of cancer cells

Life Sci. 2013 Feb 7;92(2):154-60. doi: 10.1016/j.lfs.2012.11.009. Epub 2012 Nov 28.

Abstract

Aims: Alpinia katsumadai was recently found in our previous study to have anti-migratory and anti-invasion activities against HT-1080 cells. However, the study did not demonstrate the exact component of Alpinia katsumadai with anti-migratory and anti-invasive activities. We tested the effects and relevant mechanism of cardamonin (CDN) on the migration and invasion of cancer cells.

Main methods: Migration and invasion of cancer cells were measured using multi-well chambers. Zymography and Western blots were used to examine the effects of CDN on the activities of matrix metalloproteinases (MMPs) and expression of transglutaminase-2 (Tgase-2).

Key findings: CDN, but not alpinetin, dose-dependently suppressed the migration and 12-O-tetradecanoylphorbol-13-acetate (TPA)-induced invasion of HT-1080 sarcoma cells. CDN suppressed the expression of Tgase-2, MMP-2, NF-κB and MMP-9 in HT-1080 cells, and suppressed MMP-2 and MMP-9 activities. Gene silencing of Tgase-2 suppressed the migration and invasion of HT-1080 cells and suppressed the activities of MMP-2 and MMP-9. Migration of various cancer cells having high levels of Tgase-2 were also inhibited by CDN. CDN and Alpinia katsumadai extracts also directly inhibited the activity of Tgase-2.

Significance: CDN inhibits migration of several cancer cell lines expressing Tgase-2 via suppression of Tgase-2 expression and inhibition of Tgase-2 activity. The finding that CDN has Tgase-2 inhibitory activity will give us a new scaffold or clue of pharmacophore for the development of more effective Tgase-2 inhibitors.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cell Line, Tumor
  • Cell Migration Assays
  • Cell Movement / drug effects*
  • Cell Movement / physiology
  • Chalcones / pharmacology*
  • Dose-Response Relationship, Drug
  • GTP-Binding Proteins / biosynthesis
  • GTP-Binding Proteins / drug effects*
  • GTP-Binding Proteins / physiology
  • Gene Expression Regulation, Neoplastic / drug effects
  • Gene Expression Regulation, Neoplastic / physiology
  • Gene Silencing / drug effects
  • Gene Silencing / physiology
  • Humans
  • Matrix Metalloproteinase 2 / biosynthesis
  • Matrix Metalloproteinase 2 / drug effects
  • Matrix Metalloproteinase 2 / physiology
  • Matrix Metalloproteinase 9 / biosynthesis
  • Matrix Metalloproteinase 9 / drug effects
  • Matrix Metalloproteinase 9 / physiology
  • NF-kappa B / biosynthesis
  • NF-kappa B / drug effects
  • NF-kappa B / physiology
  • Neoplasm Invasiveness / physiopathology*
  • Neoplasm Invasiveness / prevention & control
  • Protein Glutamine gamma Glutamyltransferase 2
  • Transglutaminases / biosynthesis
  • Transglutaminases / drug effects*
  • Transglutaminases / physiology

Substances

  • Chalcones
  • NF-kappa B
  • Protein Glutamine gamma Glutamyltransferase 2
  • Transglutaminases
  • Matrix Metalloproteinase 2
  • Matrix Metalloproteinase 9
  • GTP-Binding Proteins
  • cardamonin