Dynamics of nonclassical light from a single solid-state quantum emitter

Phys Rev Lett. 2012 Oct 19;109(16):163601. doi: 10.1103/PhysRevLett.109.163601. Epub 2012 Oct 18.

Abstract

We measure the dynamics of a nonclassical optical field using two-time second-order correlations in conjunction with pulsed excitation. The technique quantifies single-photon purity and coherence during the excitation-decay cycle of an emitter, illustrated here using a quantum dot. We observe that for certain pump wavelengths, photons detected early in the cycle have reduced single-photon purity and coherence compared to those detected later. A model indicates that the single-photon purity dynamics are due to exciton recapture after initial emission and within the same pulse cycle.