Copper catalyzed β-difluoroacetylation of dihydropyrans and glycals by means of direct C-H functionalization

Org Lett. 2013 Jul 5;15(13):3428-31. doi: 10.1021/ol401483j. Epub 2013 Jun 21.

Abstract

A copper catalyzed direct functionalization of dihydropyrans and glycals has been developed. This method affords a new and straightforward access to C-2-CF2 dihydropyrans and glycosides in a single step starting from readily available starting materials. This new copper based catalytic system, probably involving a Cu(III) species as supported by experiments, allows the formation of the valuable fluorinated glycosides in good yields.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalysis
  • Copper / chemistry*
  • Glycosides / chemistry*
  • Hydrocarbons, Fluorinated / chemistry*
  • Hydrogen Bonding
  • Molecular Structure
  • Pyrans / chemistry*

Substances

  • Glycosides
  • Hydrocarbons, Fluorinated
  • Pyrans
  • Copper