Efficient blind spectral unmixing of fluorescently labeled samples using multi-layer non-negative matrix factorization

PLoS One. 2013 Nov 8;8(11):e78504. doi: 10.1371/journal.pone.0078504. eCollection 2013.

Abstract

The ample variety of labeling dyes and staining methods available in fluorescence microscopy has enabled biologists to advance in the understanding of living organisms at cellular and molecular level. When two or more fluorescent dyes are used in the same preparation, or one dye is used in the presence of autofluorescence, the separation of the fluorescent emissions can become problematic. Various approaches have been recently proposed to solve this problem. Among them, blind non-negative matrix factorization is gaining interest since it requires little assumptions about the spectra and concentration of the fluorochromes. In this paper, we propose a novel algorithm for blind spectral separation that addresses some of the shortcomings of existing solutions: namely, their dependency on the initialization and their slow convergence. We apply this new algorithm to two relevant problems in fluorescence microscopy: autofluorescence elimination and spectral unmixing of multi-labeled samples. Our results show that our new algorithm performs well when compared with the state-of-the-art approaches for a much faster implementation.

Publication types

  • Clinical Trial
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Algorithms*
  • Female
  • Fluorescent Dyes / chemistry*
  • Humans
  • Image Processing, Computer-Assisted*
  • Male
  • Microscopy, Fluorescence / methods
  • Models, Theoretical*
  • Neoplasms* / metabolism
  • Neoplasms* / pathology
  • Staining and Labeling*

Substances

  • Fluorescent Dyes

Grants and funding

This project was partially funded by the “UTE Project CIMA,” the subprogram for unique strategic projects of the Spanish Science and Innovation Ministry (MCIIN PSS-010000-2008-2) and projects MICINN TEC2005-04732, MICINN DPI2009-14115-C03-03 and MINECO DPI2012-38090-C03-02. TP had a predoctoral fellowship granted by MICINN. AMB holds a Ramón y Cajal fellowship granted by the Spanish Ministry of Science and Innovation. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.