Two-dimensional 1H-NMR study of synthetic peptides containing the main immunogenic region of the Torpedo acetylcholine receptor

Biopolymers. 1989 Jan;28(1):465-78. doi: 10.1002/bip.360280141.

Abstract

A comparative 1H-NMR spectral study of a synthetic decapeptide containing the main immunogenic region of the Torpedo acetylcholine receptor (AChR; WNPADYGGIK, representing the alpha 67-76 fragment of Torpedo AChR) with four analogous peptides (WNP3-D5YGGIK, WNPAA5YGGIK, WNPADYGGA9K, and WNPD4DYGGV9K) has been carried out in dimethyl sulfoxide. One- and two-dimensional nmr experiments [correlated spectroscopy (COSY), relayed COSY, and phase-sensitive nuclear Overhauser enhancement spectroscopy (NOESY)] were performed to obtain complete assignments of the proton resonances. The presence of strong and multiple short- and long-range NOEs, and especially a strong long-range NOE between the two Asn2-C alpha H and Gly7-C alpha H protons, argues in favor of a rigid folded structure in all five cases. Temperature dependence measurements indicate the existence of three intramolecular interactions involving the Asp3, Gly8, and Lys10 amide protons.

MeSH terms

  • Amino Acid Sequence
  • Epitopes*
  • Hydrogen
  • Magnetic Resonance Spectroscopy / methods
  • Molecular Sequence Data
  • Oligopeptides* / chemical synthesis
  • Protein Conformation
  • Receptors, Cholinergic* / immunology

Substances

  • Epitopes
  • Oligopeptides
  • Receptors, Cholinergic
  • Hydrogen