Thermodynamics of halogen bonded monolayer self-assembly at the liquid-solid interface

Chem Commun (Camb). 2014 Nov 14;50(88):13465-8. doi: 10.1039/c4cc06251e.

Abstract

Monolayer self-assembly of a hexabrominated, three-fold symmetric aromatic molecule is studied at the heptanoic acid-graphite interface. Thermodynamical insights are obtained from an adapted Born-Haber cycle that is utilized to derive the overall enthalpy change including solvent effects. Comparison with theoretical entropy estimates suggests a minor influence of solvation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Graphite / chemistry*
  • Halogens / chemistry*
  • Heptanoic Acids / chemistry*
  • Quartz Crystal Microbalance Techniques
  • Solvents / chemistry
  • Temperature
  • Thermodynamics

Substances

  • Halogens
  • Heptanoic Acids
  • Solvents
  • Graphite