Effects of oil pipeline explosion on ambient particulate matter and their associated polycyclic aromatic hydrocarbons

Environ Pollut. 2015 Jan:196:440-9. doi: 10.1016/j.envpol.2014.11.012.

Abstract

Effects of the oil pipeline explosion on PM(2.5)-associated polycyclic aromatic hydrocarbons (PAHs) and their substituted (alkylated, nitrated, oxygenated, hydroxyl and chlorinated) derivatives are assessed near the accident scene of Qingdao, China. Compared with those in TSP-PM(2.5), gaseous phase, burn residue and unburned crude oil, eighty-nine PAHs in PM(2.5) are identified and quantified to investigate the composition, temporal and spatial distribution, and sources. The concentrations of PM(2.5)-associated parent PAHs increase approximately seven times from the non-explosion samples to the explosion samples (mean ± standard deviation: 112 ± 2 vs 764 ± 15 ng/m(3)), while some substituted products (nitro- and oxy-) increase by two orders of magnitude (3117 ± 156 pg/m(3) vs 740 ± 37 ng/m(3)). The toxicity evaluation indicates the BaP equivalent concentrations (based on the US EPA's toxicity factors) in PM(2.5) are much higher than those in the other phases, especially for a long duration after the tragic accident.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Air Pollutants / analysis*
  • China
  • Environmental Monitoring*
  • Explosions
  • Particulate Matter / analysis*
  • Petroleum Pollution*
  • Polycyclic Aromatic Hydrocarbons / analysis*

Substances

  • Air Pollutants
  • Particulate Matter
  • Polycyclic Aromatic Hydrocarbons