Room-temperature voltage tunable phonon thermal conductivity via reconfigurable interfaces in ferroelectric thin films

Nano Lett. 2015 Mar 11;15(3):1791-5. doi: 10.1021/nl504505t. Epub 2015 Feb 20.

Abstract

Dynamic control of thermal transport in solid-state systems is a transformative capability with the promise to propel technologies including phononic logic, thermal management, and energy harvesting. A solid-state solution to rapidly manipulate phonons has escaped the scientific community. We demonstrate active and reversible tuning of thermal conductivity by manipulating the nanoscale ferroelastic domain structure of a Pb(Zr0.3Ti0.7)O3 film with applied electric fields. With subsecond response times, the room-temperature thermal conductivity was modulated by 11%.

Keywords: Thermal conductivity; ferroelectric; nano domain; time domain thermoreflectance; tunable.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Electromagnetic Fields
  • Materials Testing
  • Membranes, Artificial*
  • Metal Nanoparticles / chemistry*
  • Metal Nanoparticles / radiation effects*
  • Metal Nanoparticles / ultrastructure
  • Radiation Dosage
  • Temperature
  • Thermal Conductivity*
  • Vibration

Substances

  • Membranes, Artificial