Overexpression and characterization of a Ca(2+) activated thermostable β-glucosidase with high ginsenoside Rb1 to ginsenoside 20(S)-Rg3 bioconversion productivity

J Ind Microbiol Biotechnol. 2015 Jun;42(6):839-50. doi: 10.1007/s10295-015-1608-7. Epub 2015 Apr 3.

Abstract

The thermostable β-glucosidase gene from Thermotoga petrophila DSM 13995 was cloned and overexpressed in Escherichia coli. The activity of the recombinant β-glucosidase was 21 U/mL in the LB medium. Recombinant β-glucosidase was purified, and its molecular weight was approximately 81 kDa. The optimal activity was at pH 5.0 and 90 °C, and the thermostability of the enzyme was improved by Ca(2+). The β-glucosidase had high selectivity for cleaving the outer and inner glucopyranosyl moieties at the C-20 carbon of ginsenoside Rb1, which produced the pharmacologically active minor ginsenoside 20(S)-Rg3. In a reaction at 90 °C and pH 5.0, 10 g/L of ginsenoside Rb1 was transformed into 6.93 g/L of Rg3 within 90 min, with a corresponding molar conversion of 97.9%, and Rg3 productivity of 4620 mg/L/h. This study is the first report of a GH3-family enzyme that used Ca(2+) to improve its thermostability, and it is the first report on the high substrate concentration bioconversion of ginsenoside Rb1 to ginsenoside 20(S)-Rg3 by using thermostable β-glucosidase under high temperature.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biotransformation
  • Calcium / metabolism*
  • Calcium / pharmacology
  • Enzyme Activation
  • Enzyme Stability / drug effects
  • Escherichia coli / genetics
  • Ginsenosides / metabolism*
  • Gram-Negative Anaerobic Straight, Curved, and Helical Rods / enzymology
  • Gram-Negative Anaerobic Straight, Curved, and Helical Rods / genetics
  • Hydrogen-Ion Concentration
  • Molecular Weight
  • Temperature
  • beta-Glucosidase / chemistry
  • beta-Glucosidase / genetics*
  • beta-Glucosidase / isolation & purification
  • beta-Glucosidase / metabolism*

Substances

  • Ginsenosides
  • ginsenoside Rb1
  • beta-Glucosidase
  • Calcium