Targeting the Two Oncogenic Functional Sites of the HPV E6 Oncoprotein with a High-Affinity Bivalent Ligand

Angew Chem Int Ed Engl. 2015 Jun 26;54(27):7958-62. doi: 10.1002/anie.201502646. Epub 2015 May 27.

Abstract

The E6 oncoproteins of high-risk mucosal (hrm) human papillomaviruses (HPVs) contain a pocket that captures LxxLL motifs and a C-terminal motif that recruits PDZ domains, with both functions being crucial for HPV-induced oncogenesis. A chimeric protein was built by fusing a PDZ domain and an LxxLL motif, both known to bind E6. NMR spectroscopy, calorimetry and a mammalian protein complementation assay converged to show that the resulting PDZ-LxxLL chimera is a bivalent nanomolar ligand of E6, while its separated PDZ and LxxLL components are only micromolar binders. The chimera binds to all of the hrm-HPV E6 proteins tested but not to low-risk mucosal or cutaneous HPV E6. Adenovirus-mediated expression of the chimera specifically induces the death of HPV-positive cells, concomitant with increased levels of the tumour suppressor P53, its transcriptional target p21, and the apoptosis marker cleaved caspase 3. The bifunctional PDZ-LxxLL chimera opens new perspectives for the diagnosis and treatment of HPV-induced cancers.

Keywords: antitumor agents; human papillomavirus; inhibitors; peptides; protein engineering.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenoviridae / genetics
  • Amino Acid Motifs
  • Binding Sites
  • Cell Death
  • Cell Line
  • DNA-Binding Proteins / chemistry
  • DNA-Binding Proteins / metabolism*
  • Gene Expression
  • HeLa Cells
  • Human papillomavirus 16 / chemistry
  • Human papillomavirus 16 / metabolism*
  • Human papillomavirus 18 / chemistry
  • Human papillomavirus 18 / metabolism*
  • Humans
  • Ligands
  • Models, Molecular
  • Neoplasms / metabolism
  • Neoplasms / therapy
  • Neoplasms / virology*
  • Oncogene Proteins, Viral / chemistry
  • Oncogene Proteins, Viral / metabolism*
  • PDZ Domains
  • Papillomavirus Infections / metabolism
  • Papillomavirus Infections / therapy
  • Papillomavirus Infections / virology*
  • Protein Binding
  • Recombinant Fusion Proteins / chemistry
  • Recombinant Fusion Proteins / genetics
  • Recombinant Fusion Proteins / metabolism*
  • Recombinant Fusion Proteins / pharmacology
  • Repressor Proteins / chemistry
  • Repressor Proteins / metabolism*
  • Tumor Suppressor Protein p53 / metabolism

Substances

  • DNA-Binding Proteins
  • E6 protein, Human papillomavirus type 16
  • E6 protein, Human papillomavirus type 18
  • Ligands
  • Oncogene Proteins, Viral
  • Recombinant Fusion Proteins
  • Repressor Proteins
  • Tumor Suppressor Protein p53