Hybrid pulmonary surfactant-coated nanogels mediate efficient in vivo delivery of siRNA to murine alveolar macrophages

J Control Release. 2015 Nov 10:217:53-63. doi: 10.1016/j.jconrel.2015.08.030. Epub 2015 Aug 22.

Abstract

The local delivery of small interfering RNA (siRNA) to the lungs may provide a therapeutic solution to a range of pulmonary disorders. Resident alveolar macrophages (rAM) in the bronchoalveolar lumen play a critical role in lung inflammatory responses and therefore constitute a particularly attractive target for siRNA therapeutics. However, achieving efficient gene silencing in the lung while avoiding pulmonary toxicity requires appropriate formulation of siRNA in functional nanocarriers. In this study, we evaluated pulmonary surfactant-coated dextran nanogels for the delivery of siRNA to rAM upon pharyngeal aspiration in BALB/c mice. Both the surfactant-coated and uncoated nanogels achieved high levels of siRNA uptake in rAM, yet only the surfactant-coated formulation could significantly reduce gene expression on the protein level. Surfactant-coated nanogels induced a profound downregulation of target mRNA levels, reaching 70% knockdown with ~1mgkg(-1) siRNA dose. In addition, only mild acute pro-inflammatory cytokine and chemokine responses were detected one day after nanoparticle aspiration, accompanied by a moderate neutrophil infiltration in the bronchoalveolar lumen. The latter could be substantially reduced by removal of excess surfactant from the formulation. Overall, our hybrid core-shell nanoparticles have demonstrated safe and effective siRNA delivery to rAM, providing a new therapeutic approach for treatment of inflammatory pathologies in the lung.

Keywords: Dextran nanogel; In vivo test; Macrophage; Pulmonary delivery; Pulmonary surfactant; siRNA.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Bronchoalveolar Lavage Fluid / chemistry
  • Bronchoalveolar Lavage Fluid / cytology
  • Cell Count
  • Cytokines / metabolism
  • Dextrans / chemistry
  • Female
  • Gels
  • Gene Silencing
  • Leukocyte Common Antigens / genetics*
  • Leukocyte Common Antigens / metabolism
  • Macrophages, Alveolar / metabolism*
  • Mice, Inbred BALB C
  • Nanoparticles / administration & dosage*
  • Nanoparticles / chemistry
  • Pulmonary Surfactants / administration & dosage*
  • Pulmonary Surfactants / chemistry
  • RNA, Small Interfering / administration & dosage*

Substances

  • Cytokines
  • Dextrans
  • Gels
  • Pulmonary Surfactants
  • RNA, Small Interfering
  • Leukocyte Common Antigens