Creation of X-Ray Transparency of Matter by Stimulated Elastic Forward Scattering

Phys Rev Lett. 2015 Sep 4;115(10):107402. doi: 10.1103/PhysRevLett.115.107402. Epub 2015 Sep 4.

Abstract

X-ray absorption by matter has long been described by the famous Beer-Lambert law. Here, we show how this fundamental law needs to be modified for high-intensity coherent x-ray pulses, now available at x-ray free electron lasers, due to the onset of stimulated elastic forward scattering. We present an analytical expression for the modified polarization-dependent Beer-Lambert law for the case of resonant core-to-valence electronic transitions and incident transform limited x-ray pulses. Upon transmission through a solid, the resonant absorption and dichroic contrasts are found to vanish with increasing x-ray intensity, with the stimulation threshold lowered by orders of magnitude through a resonant superradiantlike effect. Our results have broad implications for the study of matter with x-ray lasers.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Circular Dichroism / methods
  • Cobalt / chemistry
  • Elasticity
  • Iron / chemistry
  • Magnetics / methods
  • Models, Theoretical*
  • Nickel / chemistry
  • X-Ray Diffraction*

Substances

  • Cobalt
  • Nickel
  • Iron