Drug delivery of oral anti-cancer fluoropyrimidine agents

Expert Opin Drug Deliv. 2017 Dec;14(12):1355-1366. doi: 10.1080/17425247.2017.1316260. Epub 2017 Apr 11.

Abstract

Sixty years since its introduction, 5-FU still forms the core of chemotherapy regimens for many types of malignancies. 5-FU is a time-dependent drug but is rapidly degraded in plasma by dihydropyrimidine dehydrogenase (DPD). Although originally developed in an intravenous form, 5-FU oral prodrugs were developed with the goal of improving efficacy and minimizing toxicity as well as to capitalize on the advantages of oral drug administration. The inactive 5-FU prodrug is gradually converted into the active form in the systemic circulation. UFT, S-1, and capecitabine are oral 5-FU prodrugs currently in clinical use. However, the efficacy of 5-FU can be further improved by its combination with DPD inhibitors and biochemical modulators, such as uracil and leucovorin, in addition to modifying administration schedules. Areas covered: We focused on the drug delivery of oral 5-FU prodrugs, their pharmacokinetics, and the development of DPD inhibitors. Since oral 5-FU prodrugs have been formulated into combination drugs, we also discussed the regulatory approval of combination drugs. Expert opinion: Many regimens that include intravenously administered 5-FU can be replaced by oral 5-FU prodrugs. Patients would benefit from development of combination 5-FU oral prodrug formulations and its associated path through the combination drug regulatory approval process.

Keywords: Anti-cancer fluoropyrimidine agent; FDA approval; dihydropyrimidine dehydrogenase inhibitor; fixed-dose combination drug; oral administration; prodrug.

Publication types

  • Review

MeSH terms

  • Administration, Intravenous
  • Administration, Oral
  • Antimetabolites, Antineoplastic / administration & dosage*
  • Antimetabolites, Antineoplastic / therapeutic use
  • Antineoplastic Agents / administration & dosage*
  • Antineoplastic Agents / therapeutic use
  • Antineoplastic Combined Chemotherapy Protocols / administration & dosage
  • Dihydrouracil Dehydrogenase (NADP) / antagonists & inhibitors
  • Drug Delivery Systems / methods*
  • Enzyme Inhibitors / administration & dosage
  • Fluorouracil / administration & dosage*
  • Fluorouracil / therapeutic use
  • Humans
  • Neoplasms / drug therapy*
  • Prodrugs / administration & dosage
  • Pyrimidines

Substances

  • Antimetabolites, Antineoplastic
  • Antineoplastic Agents
  • Enzyme Inhibitors
  • Prodrugs
  • Pyrimidines
  • Dihydrouracil Dehydrogenase (NADP)
  • Fluorouracil