Bioluminescent Turn-On Probe for Sensing Hypochlorite in Vitro and in Tumors

Anal Chem. 2017 Jun 6;89(11):5693-5696. doi: 10.1021/acs.analchem.7b01103. Epub 2017 May 10.

Abstract

Hypochlorite (ClO-) is one of the most important reactive oxygen species but using a BL probe for its selective detection (or imaging) still remains challenging. Herein, we report a latent BL probe benzoylhydrazine luciferin (1) for highly selective detection of ClO- in vitro and imaging ClO- in living cells and tumors. In vitro tests indicated that 1 could be applied for highly selective detection of ClO- within the range of 0-62.5 μM with a limit of detection of 0.705 μM. Using these unique features of 1, we successfully applied it to image ClO- in living cells and tumors. We envision that probe 1 might be applied to elucidate the biological roles of ClO- in wider physiological and pathological processes in the near future.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Firefly Luciferin
  • Hydrazines
  • Hypochlorous Acid / analysis*
  • Limit of Detection
  • Luminescent Agents
  • Luminescent Measurements / methods*
  • Molecular Imaging / methods*
  • Neoplasms / chemistry*
  • Oxidants

Substances

  • Hydrazines
  • Luminescent Agents
  • Oxidants
  • Firefly Luciferin
  • Hypochlorous Acid
  • benzoylhydrazine