A novel biodegradation pathway of the endocrine-disruptor di(2-ethyl hexyl) phthalate by Pleurotus ostreatus based on quantum chemical investigation

Ecotoxicol Environ Saf. 2018 Jan:147:494-499. doi: 10.1016/j.ecoenv.2017.09.004. Epub 2017 Sep 14.

Abstract

Di(2-ethyl hexyl) phthalate (DEHP) is a plasticizer that interfere with endocrine systems in mammals. Growth parameters for Pleurotus ostreatus grown on media containing glucose and different concentrations of DEHP (0, 500 and 1000mg/L) were evaluated. The highest biomass production was observed in medium supplemented with 1000mg of DEHP/L. Half-life of DEHP biodegradation, biodegradation constant of DEHP, and percentage of removal efficiency (%E) were also determined. P. ostreatus degraded 100% of DEHP after 504h. %E was 99.3% and 98.4% for 500 and 1000mg of DEHP/L, respectively. Intermediate compounds of biodegraded DEHP were identified by GC-MS and a DEHP biodegradation pathway was proposed using quantum chemical investigation. DEHP might be metabolized through three pathways; a de-esterification pathway, an oxidation pathway and an oxidation-hydrolysis pathway, forming phthalic acid, acetic acid and butanediol, respectively. P. ostreatus degrades and uses (as carbon and energy source) high concentrations of DEHP.

Keywords: Biodegradation; Di(2-ethylhexyl) phthalate; Pleurotus ostreatus; Removal efficiency.

MeSH terms

  • Animals
  • Biodegradation, Environmental
  • Biomass
  • Biotransformation
  • Diethylhexyl Phthalate / analysis*
  • Diethylhexyl Phthalate / metabolism
  • Endocrine Disruptors / analysis*
  • Endocrine Disruptors / metabolism
  • Gas Chromatography-Mass Spectrometry
  • Half-Life
  • Plasticizers / analysis*
  • Plasticizers / metabolism
  • Pleurotus / growth & development
  • Pleurotus / metabolism*

Substances

  • Endocrine Disruptors
  • Plasticizers
  • Diethylhexyl Phthalate