Mirror image pairs of cyclic hexapeptides have different oral bioavailabilities and metabolic stabilities

Chem Commun (Camb). 2019 Nov 18;55(89):13362-13365. doi: 10.1039/c9cc06234c. Epub 2019 Oct 21.

Abstract

Rule-of-five parameters and membrane permeabilities have been routinely used to guide development of orally bioavailabile drugs. Here we compare enantiomeric pairs of cyclic hexapeptides with identical rule-of-five parameters and membrane permeabilities. For each enantiomeric pair, the isomer with more l- than d-amino acids is much more orally bioavailable in rats, more metabolically stable to rat liver microsomes, and cleared more slowly in vivo.

MeSH terms

  • Administration, Oral
  • Animals
  • Biological Availability
  • Microsomes, Liver / chemistry
  • Microsomes, Liver / metabolism
  • Molecular Conformation
  • Peptides, Cyclic / administration & dosage
  • Peptides, Cyclic / metabolism*
  • Peptides, Cyclic / pharmacokinetics*
  • Rats
  • Stereoisomerism

Substances

  • Peptides, Cyclic