Crystal structures of 2,3,7,8,12,13,17,18-octa-bromo-5,10,15,20-tetra-kis-(penta-fluoro-phen-yl)porphyrin as the chloro-form monosolvate and tetra-hydro-furan monosolvate

Acta Crystallogr E Crystallogr Commun. 2020 Jan 17;76(Pt 2):214-220. doi: 10.1107/S2056989020000432. eCollection 2020 Feb 1.

Abstract

The crystal structures of the title compounds, two solvates (CHCl3 and THF) of a symmetric and highly substituted porphyrin, C44H2Br8F20N4 or OBrTPFPP, are described. These structures each feature a non-planar porphyrin ring, exhibiting a similar conformation of the strained ring independent of solvent identity. These distorted porphyrins are able to form hydrogen bonds and sub-van der Waals halogen inter-actions with enclathrated solvent; supra-molecular inter-actions of proximal macrocycles are additionally affected by solvent choice. The crystal studied for compound 1·CHCl3 was refined as an inversion twin. One penta-fluoro-phenyl group was modelled as disordered over two sites [occupancy ratio = 0.462 (7):0.538 (7)]. The chloro-form solvate was also modelled as disordered over two orientations [occupancy ratio = 0.882 (7): 0.118 (7).

Keywords: crystal structure; halogenated porphyrins; non-planar porphyrins; solvent inter­actions; symmetrical porphyrins.

Grants and funding

This work was funded by Science Foundation Ireland grant SFI, IvP 13/IA/1894. Horizon 2020 grant FET-OPEN grant agreement o. 828779.