Poly-ε-caprolactone (PCL)/poly-l-lactic acid (PLLA) nanofibers loaded by nanoparticles-containing TGF-β1 with linearly arranged transforming structure as a scaffold in cartilage tissue engineering

J Biomed Mater Res A. 2023 Dec;111(12):1838-1849. doi: 10.1002/jbm.a.37574. Epub 2023 Jul 3.

Abstract

This study aimed to present a novel three-dimensional nanocomposite scaffold using poly-ε-caprolactone (PCL), containing transforming growth factor-beta 1 (TGF-β1)-loaded chitosan-dextran nanoparticles and poly-l-lactic acid (PLLA), to make use of nanofibers and nanoparticles simultaneously. The electrospinning method fabricated a bead-free semi-aligned nanofiber composed of PLLA, PCL, and chitosan-dextran nanoparticles containing TGF-β1. A biomimetic scaffold was constructed with the desired mechanical properties, high hydrophilicity, and high porosity. Transmission electron microscopy findings showed a linear arrangement of nanoparticles along the core of fibers. Based on the results, burst release was not observed. The maximum release was achieved within 4 days, and sustained release was up to 21 days. The qRT-PCR results indicated an increase in the expression of aggrecan and collagen type Ι genes compared to the tissue culture polystyrene group. The results indicated the importance of topography and the sustained release of TGF-β1 from bifunctional scaffolds in directing the stem cell fate in cartilage tissue engineering.

Keywords: PCL/PLLA nanofiber; cartilage tissue engineering; chitosan-dextran nanoparticle; electrospinning; mesenchymal stem cell; topography of nanoparticles.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cartilage
  • Chitosan* / chemistry
  • Delayed-Action Preparations
  • Dextrans
  • Nanofibers* / chemistry
  • Nanoparticles* / chemistry
  • Polyesters / chemistry
  • Tissue Engineering / methods
  • Tissue Scaffolds / chemistry
  • Transforming Growth Factor beta1

Substances

  • poly(lactide)
  • caprolactone
  • Transforming Growth Factor beta1
  • Delayed-Action Preparations
  • Chitosan
  • Dextrans
  • Polyesters