A portable europium complex-loaded fluorescent test paper combined with smartphone analysis for the on-site and visual detection of mancozeb in food samples

Food Chem. 2024 Nov 15:458:140311. doi: 10.1016/j.foodchem.2024.140311. Epub 2024 Jul 2.

Abstract

The on-site detection of mancozeb in food samples holds immense value for food safety. A red-fluorescent europium complex (Eu-PYDC-Phen) has been prepared and employed as a fluorescence probe for mancozeb detection. The optimized probe suspension exhibits excellent detection performances, including a wide linear range (0-0.24 mM), low detection limit (65 nM), rapid response (2 mins) and high selectivity. Moreover, a portable detection platform was carefully designed, integrating the Eu-PYDC-Phen-based fluorescent test strips with smartphone color recognition software. This innovative platform enables visual and on-site detection of mancozeb in tomato, apple, and lettuce, achieving satisfactory recovery rates (90.34 to 106.50%). Furthermore, the integration of machine learning techniques based on hierarchical clustering algorithm has the potential to further improve the prediction and decision-making efficiency in mancozeb detection. This work provides an economical, convenient, and reliable strategy for on-site detection of pesticide in agricultural products, thereby making a meaningful contribution to food safety.

Keywords: Europium complex; Mancozeb; On-site detection; Paper-based probe; Smartphone.

Publication types

  • Evaluation Study

MeSH terms

  • Europium* / chemistry
  • Fluorescent Dyes / chemistry
  • Food Analysis / instrumentation
  • Food Analysis / methods
  • Food Contamination* / analysis
  • Lactuca / chemistry
  • Limit of Detection
  • Malus / chemistry
  • Maneb* / analysis
  • Paper
  • Smartphone*
  • Solanum lycopersicum / chemistry
  • Spectrometry, Fluorescence / instrumentation
  • Spectrometry, Fluorescence / methods
  • Zineb* / analysis

Substances

  • mancozeb
  • Zineb
  • Maneb
  • Europium
  • Fluorescent Dyes