Research on the Dynamic Spreading and Wettability Characteristics of Droplets on Coal Dust

ACS Omega. 2024 Nov 11;9(47):46751-46761. doi: 10.1021/acsomega.4c00881. eCollection 2024 Nov 26.

Abstract

The dynamics of droplets spreading on surfaces have been extensively studied across various influencing factors, necessitating an exploration of their effect on wettability. Herein, the specific composition, size distribution, and contact angle of the coal dust preparation were characterized by a series of experiments to determine the conditions for the simulation. Meanwhile, the multiphase volume of the fluid method was implemented in the simulations, predicated on appropriate boundary conditions, and verified by a mesh independence test. The findings confirmed that the numerical approach for contact angle validation had a minor deviation, making it suitable for multiphase interface tracking. Besides, the typical wetting pattern of droplets was hereby identified into three stages, including the moving stage (stage I), the periodic wetting stage (stage II), and the balancing stage (stage III). The initial diameter could effectively increase the coverage area and spreading time for stage II. Obviously, the first amplitude of first maximum spreading diameter (D max-1) significantly increased with higher impact velocities, corresponding to an increase in kinetic energy. Despite the significant spreading effect of the falling height mainly on D max-1 and contact time, the increased trend of wetting efficiency was not obvious. However, the spreading factor and wetting efficiency decreased with increased roughness height. Finally, the difference in spreading wettability was illustrated based on the spreading wetting mechanism. The wetting efficiency of droplets on coal dust was remarkably influenced by the dynamic spreading behaviors of droplets. Overall, the findings from this study offer insights into the extent of spreading wetting that occurs before a droplet reaches an equilibrium state.