[Distribution and Source-specific Ecological Risk Analysis of Soil Heavy Metals in South Hunan Province]

Huan Jing Ke Xue. 2025 Jan 8;46(1):430-441. doi: 10.13227/j.hjkx.202401210.
[Article in Chinese]

Abstract

To identify the spatial distribution patterns and assess the ecological risks associated with soil heavy metal pollution in the southern region of Hunan Province, a total of 362 surface soil samples were collected from the studied area. This study employed multivariate statistics and geographic information systems (GIS) to investigate the spatial distribution pattern of soil metals (Cd, Hg, As, Pb, Zn, Ni, Mn, Tl, and Sb). Furthermore, the pollution sources and source-specific ecological risk of heavy metals were quantified by combining the positive matrix factorization (PMF) model and the comprehensive ecological risk index model. The results suggested that the mean concentration of soil metals in the study area exceeded the mean background values. Specifically, Cd, Hg, Pb, and Sb showed significant pollution levels and substantial spatial variability, with their concentrations reaching the background values by factors of 8.31, 9.12, 5.09, and 2.79, respectively. The spatial distribution of these heavy metals exhibited discernible patterns, with a higher concentration observed in western Chenzhou and a noticeable trend of increasing concentrations from the central region towards the periphery. The clusters with high concentrations of heavy metals were predominantly situated near industrial zones engaged in black metal smelting and processing and nonferrous metal mining and processing enterprises. Source apportionment indicated that the primary sources of soil heavy metals in the area were industrial activities associated with black metal mining and metallurgy (29.06%), atmospheric deposition (22.05%), nonferrous metal mining and processing (20.65%), a combination of industrial and transportation sources (14.73%), and natural sources (13.50%). Moreover, the source-ecological risk assessment model specifically identified Cd and Hg as crucial elements requiring prioritized control measures to mitigate soil ecological risks. Industrial activities, including black metal smelting and processing and atmospheric deposition sources, were identified as the priority sources for health risks in the study region. These results provide an important theoretical basis for the development of effective strategies aimed at managing and diminishing the risks associated with heavy metal contamination in the southern region of Hunan Province.

Keywords: ecological risk; heavy metals; soil; source apportionment; spatial distribution.

Publication types

  • English Abstract