Pseudospecific docking surfaces on electron transfer proteins as illustrated by pseudoazurin, cytochrome c550 and cytochrome cd1 nitrite reductase

Nat Struct Biol. 1995 Nov;2(11):975-82. doi: 10.1038/nsb1195-975.

Abstract

The structure of pseudoazurin from Thiosphaera pantotropha has been determined and compared to structures of both soluble and membrane-bound periplasmic redox proteins. The results show a matching set of unipolar, but promiscuous, docking motifs based on a positive hydrophobic surface patch on the electron shuttle proteins pseudoazurin and cytochrome c550 and a negative hydrophobic patch on the surface of their known redox partners. The observed electrostatic handedness is argued to be associated with the charge-asymmetry of the membrane-bound components of the redox chain due to von Heijne's 'positives-inside' principle. We propose a 'positives-in-between' rule for electron shuttle proteins, and expect a negative hydrophobic patch to be present on both the highest and lowest redox potential species in a series of electron carriers.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Azurin / analogs & derivatives*
  • Azurin / chemistry
  • Azurin / metabolism
  • Crystallography, X-Ray
  • Cytochrome c Group / chemistry
  • Cytochrome c Group / metabolism
  • Cytochromes / chemistry
  • Cytochromes / metabolism
  • Electron Transport*
  • Gram-Negative Chemolithotrophic Bacteria / chemistry
  • Models, Molecular
  • Nitrite Reductases / chemistry
  • Nitrite Reductases / metabolism
  • Protein Conformation

Substances

  • Cytochrome c Group
  • Cytochromes
  • pseudoazurin
  • Azurin
  • cytochrome cd1
  • cytochrome C-550
  • Nitrite Reductases