Thermostable N-carbamoyl-D-amino acid amidohydrolase: screening, purification and characterization

J Biotechnol. 1994 Nov 30;38(1):11-9. doi: 10.1016/0168-1656(94)90143-0.

Abstract

A thermostable N-carbamoyl-D-amino acid amidohydrolase was found in the cells of newly isolated bacterium. Blastobacter sp. A17p-4. The bacterium also showed D-specific hydantoinase activity. The N-carbamoyl-D-amino acid amidohydrolase activity of the cells exhibited a temperature optimum at 50-55 degrees C, and was stable up to 50 degrees C. The N-carbamoyl-D-amino acid amidohydrolase of Blastobacter sp. A17p-4 was purified to homogeneity and characterized. It has a relative molecular weight of about 120,000 and consists of three identical subunits with a relative molecular weight of about 40,000. N-Carbamoyl-D-amino acids having hydrophobic groups served as good substrates for the enzyme. It has been suggested that D-amino acid production from DL-5-substituted hydantoin involves the action of a series of enzymes involved in pyrimidine degradation, namely amide-ring opening enzyme, dihydropyrimidinase, and N-carbamoylamide hydrolyzing enzyme, beta-ureidopropionase. However, the purified enzyme did not hydrolyze beta-ureidopropionate; suggesting that the N-carbamoyl-D-amino acid amidohydrolase coexisting with D-specific hydantoinase, probably dihydropyrimidinase, in Blastobacter sp. A17p-4 is different from beta-ureidopropionase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amidohydrolases / antagonists & inhibitors
  • Amidohydrolases / isolation & purification
  • Amidohydrolases / metabolism*
  • Amino Acid Sequence
  • Chromatography, Gel
  • Electrophoresis, Polyacrylamide Gel
  • Enzyme Stability
  • Gram-Negative Bacteria / enzymology*
  • Hot Temperature
  • Molecular Sequence Data

Substances

  • Amidohydrolases
  • N-carbamoyl-D-amino acid amidohydrolase