Changing the inhibitory specificity and function of Cucurbita maxima trypsin inhibitor-V by site-directed mutagenesis

Biochem Biophys Res Commun. 1995 Feb 27;207(3):897-902. doi: 10.1006/bbrc.1995.1270.

Abstract

Cucurbita maxima trypsin inhibitor-V (CMTI-V) is also a specific inhibitor of human blood coagulation factor beta-factor XIIa. A recombinant version of CMTI-V has allowed probing of roles of individual amino acid residues including the reactive site residue, lysine (P1), by site-directed mutagenesis. The K44R showed at least a 5-fold increase in inhibitory activity toward human beta-factor XIIa, while there was no change toward bovine trypsin. This result demonstrates that beta-factor-XIIa prefers an arginine residue over lysine residue, while trypsin is non-specific to lysine or arginine in its binding pocket. On the other hand, the specificity of CMTI-V could be changed from trypsin to chymotrypsin inhibition by mutation of the P1 residue to either leucine or methionine (K44L or K44M).

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Arginine
  • Base Sequence
  • Binding Sites
  • Cattle
  • Chymotrypsin / metabolism
  • Factor XIIa / antagonists & inhibitors
  • Humans
  • Lysine
  • Molecular Sequence Data
  • Mutagenesis, Site-Directed*
  • Plant Proteins / chemistry
  • Plant Proteins / genetics
  • Plant Proteins / pharmacology*
  • Structure-Activity Relationship
  • Trypsin / metabolism
  • Trypsin Inhibitors / chemistry
  • Trypsin Inhibitors / genetics
  • Trypsin Inhibitors / pharmacology*

Substances

  • CMTI protein, Cucurbita maxima
  • Plant Proteins
  • Trypsin Inhibitors
  • Arginine
  • Chymotrypsin
  • Factor XIIa
  • Trypsin
  • Lysine