Composition and phase behaviour of polar lipids isolated from Spirulina maxima cells grown in a perdeuterated medium

Biochim Biophys Acta. 1996 Oct 23;1284(2):196-202. doi: 10.1016/s0005-2736(96)00129-0.

Abstract

The lipid composition of Spirulina maxima cells grown in a perdeuterated medium was determined by using nuclear magnetic resonance spectroscopy, fast atom-bombardment-mass spectrometry, gas chromatography-mass spectrometry as well as conventional chemical methods. The extent of deuteration was determined by mass spectrometry and was superior to 97.5%. The major lipids identified in the strain were: non-polar lipids (9%), monogalactosyldiacylglycerol (5%), digalactosyldiacylglycerol (22%), phosphatidylglycerol (31%), sulfoquinovosyldiacylglycerol (32%), phosphatidylinositol (traces). The major fatty acids were 16:0 (80%) and 18:1 (15%). These results demonstrate that the adaptation of the cells to D2O did not imply a profound modification of the lipid composition. The perdeuterated polar lipid mixture dispersed into an excess of water organises spontaneously in a lamellar phase as seen by 31P and deuterium solid state NMR and can therefore be used to prepare perdeuterated model membranes with a well defined composition. Liposomes made using these lipids have a gel to liquid-crystalline phase transition in the range 15-27 degrees C and are in a fluid L alpha phase above this temperature.

MeSH terms

  • Chromatography, DEAE-Cellulose
  • Cyanobacteria / chemistry
  • Cyanobacteria / growth & development
  • Cyanobacteria / metabolism*
  • Deuterium Oxide
  • Fatty Acids / analysis
  • Gas Chromatography-Mass Spectrometry
  • Glycolipids / chemistry
  • Glycolipids / isolation & purification
  • Glycolipids / metabolism
  • Lipid Metabolism*
  • Lipids / chemistry
  • Lipids / isolation & purification
  • Magnetic Resonance Spectroscopy
  • Radioisotope Dilution Technique
  • Spectrometry, Mass, Fast Atom Bombardment
  • Spectroscopy, Fourier Transform Infrared

Substances

  • Fatty Acids
  • Glycolipids
  • Lipids
  • Deuterium Oxide