Neurochemical and behavioral effects of ciproxifan, a potent histamine H3-receptor antagonist

J Pharmacol Exp Ther. 1998 Nov;287(2):658-66.

Abstract

Ciproxifan, i.e., cyclopropyl-(4-(3-1H-imidazol-4-yl)propyloxy) phenyl) ketone, belongs to a novel chemical series of histamine H3-receptor antagonists. In vitro, it behaved as a competitive antagonist at the H3 autoreceptor controlling [3H]histamine release from synaptosomes and displayed similar Ki values (0.5-1.9 nM) at the H3 receptor controlling the electrically-induced contraction of guinea pig ileum or at the brain H3 receptor labeled with [125I]iodoproxyfan. Ciproxifan displayed at least 3-orders of magnitude lower potency at various aminergic receptors studied in functional or binding tests. In vivo, measurement of drug plasma levels, using a novel radioreceptor assay in mice receiving ciproxifan p.o. or i.v., led to an oral bioavailability ratio of 62%. Oral administration of ciproxifan to mice enhanced by approximately 100% histamine turnover rate and steady state level of tele-methylhistamine with an ED50 of 0.14 mg/kg. Ciproxifan reversed the H3-receptor agonist induced enhancement of water consumption in rats with and ID50 of 0.09 +/- 0.04 mg/kg, i.p. In cats, ciproxifan (0.15-2 mg/kg, p.o.) induced marked signs of neocortical electroencephalogram activation manifested by enhanced fast-rhythms density and an almost total waking state. In rats, ciproxifan enhanced attention as evaluated in the five-choice task performed using a short stimulus duration. Ciproxifan appears to be an orally bioavailable, extremely potent and selective H3-receptor antagonist whose vigilance- and attention-promoting effects are promising for therapeutic applications in aging disorders.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Behavior, Animal / drug effects*
  • Cats
  • Electroencephalography
  • Female
  • Guinea Pigs
  • Histamine Antagonists / pharmacology*
  • Imidazoles / metabolism
  • Imidazoles / pharmacology*
  • Iodine Radioisotopes
  • Male
  • Methylhistamines / metabolism
  • Mice
  • Neocortex / drug effects
  • Neocortex / metabolism
  • Neocortex / physiology
  • Radioligand Assay
  • Rats
  • Rats, Wistar
  • Receptors, Histamine H3 / drug effects*
  • Receptors, Histamine H3 / metabolism

Substances

  • Histamine Antagonists
  • Imidazoles
  • Iodine Radioisotopes
  • Methylhistamines
  • Receptors, Histamine H3
  • iodoproxyfan
  • ciproxifan
  • tele-methylhistamine